Efficacious elimination of intramolecular charge transfer in perylene imide based light-harvesting antenna molecules

Rajeev K. Dubey; Damla Inan; Abbey M. Philip; Ferdinand C. Grozema; Wolter F. Jager

doi:10.1039/d0cc00335b

Efficacious elimination of intramolecular charge transfer in perylene imide based light-harvesting antenna molecules

Rajeev K. Dubey, Damla Inan, Abbey M. Philip, Ferdinand C. Grozema, Wolter F. Jager

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Abstract

Two light-harvesting antenna molecules were obtained by positioning naphthalene monoimide energy donors at the imide position, instead of the bay positions, of perylene imide energy acceptors. Such rational design resulted in a complete suppression of parasitic intramolecular charge transfer without compromising the desired ultrafast rates of excitation energy transfer.

Original language	English
Pages (from-to)	5560-5563
Journal	Chemical communications (Cambridge, England)
Volume	56
Issue number	41
DOIs	https://doi.org/10.1039/d0cc00335b
Publication status	Published - 2020

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10.1039/d0cc00335b

d0cc00335bFinal published version, 2.27 MBLicence: CC BY

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title = "Efficacious elimination of intramolecular charge transfer in perylene imide based light-harvesting antenna molecules",

abstract = "Two light-harvesting antenna molecules were obtained by positioning naphthalene monoimide energy donors at the imide position, instead of the bay positions, of perylene imide energy acceptors. Such rational design resulted in a complete suppression of parasitic intramolecular charge transfer without compromising the desired ultrafast rates of excitation energy transfer.",

author = "Dubey, {Rajeev K.} and Damla Inan and Philip, {Abbey M.} and Grozema, {Ferdinand C.} and Jager, {Wolter F.}",

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AU - Dubey, Rajeev K.

AU - Inan, Damla

AU - Philip, Abbey M.

AU - Grozema, Ferdinand C.

AU - Jager, Wolter F.

PY - 2020

Y1 - 2020

N2 - Two light-harvesting antenna molecules were obtained by positioning naphthalene monoimide energy donors at the imide position, instead of the bay positions, of perylene imide energy acceptors. Such rational design resulted in a complete suppression of parasitic intramolecular charge transfer without compromising the desired ultrafast rates of excitation energy transfer.

AB - Two light-harvesting antenna molecules were obtained by positioning naphthalene monoimide energy donors at the imide position, instead of the bay positions, of perylene imide energy acceptors. Such rational design resulted in a complete suppression of parasitic intramolecular charge transfer without compromising the desired ultrafast rates of excitation energy transfer.

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U2 - 10.1039/d0cc00335b

DO - 10.1039/d0cc00335b

M3 - Article

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SN - 1359-7345

VL - 56

SP - 5560

EP - 5563

JO - Chemical communications (Cambridge, England)

JF - Chemical communications (Cambridge, England)

IS - 41

ER -

Efficacious elimination of intramolecular charge transfer in perylene imide based light-harvesting antenna molecules

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